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The thermodynamictreatment of gasladsorbateequilibrium is in many respects analogous to that of vaporlliquid equilibrium However, the definition of a system to which the equations of thermodynamics apply presents a problem The force field of the solid adsorbent influences properties in the adjacent gas phase, but its effect decreases rapidly with distance Thus the properties of the gas change rapidly in the immediate neighborhood of the solid surface, but they do not change abruptly A region of change exists which contains gradients in the properties of the gas, but the distance into the gas phase that the solid makes its influence felt cannot be precisely established This problem is circumvented by a construct devised by J W Gibbs Imagine that the gas-phase properties extend unchanged up to the solid surface Differences between the actual and the unchanged properties can then be attributed to a mathematical surface, treated as a twodimensional phase with its own thermodynamic properties This provides not only a precisely defined surface phase to account for the singularities of the interfacial region, but it also extracts them from the three-dimensional gas phase so that it too may be treated precisely The solid, despite the influence of its force field, is presumed inert and not otherwise to participate in the gasladsorbate equilibrium Thus for purposes of thermodynamic analysis the adsorbate is treated as a two-dimensional phase, inherently an open system because it is in equilibrium with the gas phase The fundamental property relation for an open P V T system is given by Eq (112): how to use code 128 barcode font in crystal reports How to Create a Code 128 Barcode in Crystal Reports using the ...
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